Copied State-to-State Dynamical Research in the F+H2 Reaction System
State-to-State Dynamical Research in the F+H2 Reaction System
This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics ofF+H2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA)experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatususing ahydrogen atomRydberg "tagging" time-of-flight method, and presents thorough state-to-state experimental studies to addresstheabove issues. The author also describes the observation of theFeshbach resonance intheF+H2 reaction,aprecise measurement of the differential cross section intheF+HD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F*(2P1/2) intheF+D2 reaction, and exploits the breakdown of BOA in the low collision energy.
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